In 2014, T.O.P starred in the gambling film Tazza: The Hidden Card, based on the manhwa of the same name. After debuting as a furniture designer in 2015 in collaboration with Vitra, he was awarded the Visual Culture Award at the Prudential Eye Awards. Later that year, he starred in CJ E&M's web drama The Secret Message alongside Japanese actress Juri Ueno. Despite being a rapper, he sang on the single "Hi Haruka" as part of the drama's soundtrack.
In August 2014, T.O.P joined the Ice Bucket Challenge, an international campaign to develop medical treatment for Lou Gehrig's disease, also known as Amyotrophic lateral sclerosis (ALS). He made a donation to the Seungil Hope Foundation, a non-profit organization that provides aid to Lou Gehrig patients. In October 2016, in partnership with British auction house Sotheby's, he curated a collection of contemporary art as part of a special charity auction in Hong Kong. The project was named #TTTOP, and it featured 28 works by both Asian and Western artists. The auction saw a sale of more than HK$ 135 million and a portion of the proceeds was donated to the Asian Cultural Council (ACC) to support emerging Asian artists. In March 2020, T.O.P donated 100 million won to the Hope Bridge Disaster Relief Association, which announced that it would use the donation to purchase supplies for the medical teams responsible for combating the pandemic of coronavirus outbreak (COVID-19).