LiSA performed "Thrill, Risk, Heartless" as the theme song for the video game Sword Art Online: Fatal Bullet. The song was released digitally on January 9, 2018. She released two compilation albums titled LiSA Best -Day- and LiSA Best -Way- on May 9, 2018. She released a double A-sided single titled "Akai Wana (Who Loves It?) (赤い罠 (who loves it?)) / Adamas" on December 12, 2018. The song "Adamas" was used as the first opening theme to the 2018 anime series Sword Art Online: Alicization; it was released digitally on October 7, 2018. She is featured on Hiroyuki Sawano's song "Narrative", which was used as the ending theme song of the anime film Mobile Suit Gundam Narrative under the name "SawanoHiroyuki[nZk]:LiSA". Her single "Gurenge" (紅蓮華, Red Lotus), used as the first opening theme song for the 2019 anime series Demon Slayer: Kimetsu no Yaiba, was released digitally on April 22, 2019 and received a physical release on July 3, 2019. She collaborated with FictionJunction in performing the song "From the Edge" which is used as the first ending theme to Demon Slayer: Kimetsu no Yaiba. The song was released digitally on September 1, 2019. Her single "Unlasting" was released on December 11, 2019, with the title track being released digitally on October 21, 2019; "Unlasting" was used as the third ending theme to Sword Art Online: Alicization. She appeared at the 2019 Kōhaku Uta Gassen. She released her digital single "Aijō" (愛錠, Love Lock) on August 17, 2020; the song is used as the theme song for Japanese drama series 13. On October 14, 2020, she will release her fifth studio album Leo-Nine, and also a single titled "Homura" (炎, Flame); The song will be used as the theme song for the upcoming anime film Demon Slayer: Kimetsu no Yaiba the Movie: Mugen Train.