On July 28, 1961, Bond married Alice Clopton, a student at Spelman College; they divorced on November 10, 1989. They had five children: Phyllis Jane Bond-McMillan, Horace Mann Bond II, Michael Julian Bond (an Atlanta City Councilman), Jeffrey Alvin Bond and Julia Louise Bond. He married Pamela Sue Horowitz, a former SPLC staff attorney, in 1990. Bond died from complications of vascular disease on August 15, 2015, in Fort Walton Beach, Florida, at the age of 75. He is survived by his wife, his five children, his brother James and sister Jane Bond Moore, and eight grandchildren.